Ni-Electrocatalytic C(sp3)–C(sp3) Doubly Decarboxylative Coupling - Nature

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Ni-Electrocatalytic C(sp3)–C(sp3) Doubly Decarboxylative Coupling - Nature
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Nature research paper: Ni-Electrocatalytic C(sp3)–C(sp3) Doubly Decarboxylative Coupling. The reaction tolerates a range of functional groups, is scalable, and is used for the synthesis of 32 known compounds, reducing overall step-counts by 73%.

We are providing an unedited version of this manuscript to give early access to its findings. Before final publication, the manuscript will undergo further editing. Please note there may be errors present which affect the content, and all legal disclaimers apply.

From the perspective of synthesis design, this transformation could allow one to couple the most available carboxylates without regard to polarity or neighbouring functionalityIn practice, this promise is undermined by the strongly oxidative electrolytic protocol employed traditionally since the 19thereby severely limiting its scope.

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